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Speaking as a professional in the film and video world. I can tell you that you will never get them to match.
The CRT has better color and black level depth. Unless your LCD is a professional model, you won't be able to get it to match perfectly.
I used to be called in to editing and compositing rooms to do exactly the same thing. They would always want to calibrate a LCD or Plasma display bought at Best Buy to the professional CRT monitor on their desktop. You can get the the colors close, but the contrast depth would never match.
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